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Contents

  1. Defining the molecular structure
  2. Solving the Hartree-Fock equations
  3. Building the Hamiltonian
  4. Advanced features
  5. OpenFermion-PySCF backend
  6. References
  7. About the author

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  1. Demos/
  2. Quantum Chemistry/

  3. Building molecular Hamiltonians

Building molecular Hamiltonians

Alain Delgado Gran

Alain Delgado Gran

Published: August 01, 2020. Last updated: September 09, 2025.

Note

A wide variety of molecular data, including Hamiltonians, is available on the PennyLane Datasets service.

The ultimate goal of computational quantum chemistry is to unravel the quantum effects that determine the structure and properties of molecules. Reaching this goal is challenging since the characteristic energies associated with these effects, e.g., the electronic correlation energy, are typically a tiny fraction of the total energy of the molecule.

Accurate molecular properties can be computed from the wave function describing the interacting electrons in a molecule. The electronic wave function \(\Psi(r)\) satisfies the Schrödinger equation

\[H_e \Psi(r) = E \Psi(r),\]

where \(H_e\) and \(E\) denote the electronic Hamiltonian and the total energy of the molecule, respectively. When solving the latter equation, the nuclei of the molecule can be treated as point particles whose coordinates are fixed 2. In this approximation, both the total energy and the electronic Hamiltonian depend parametrically on the nuclear coordinates.

In this tutorial, you will learn how to use PennyLane to build a representation of the electronic Hamiltonian \(H_e\) that can be used to perform quantum simulations of molecules 1. First, we show how to define the structure of the molecule in terms of the symbols and the coordinates of the atoms. Next, we describe how to solve the Hartree-Fock equations for the target molecule. Finally, we discuss some advanced features that can be used to simulate more complicated systems.

Let’s get started!

Defining the molecular structure

In this example we construct the electronic Hamiltonian of the water molecule.

demos/_static/demonstration_assets/quantum_chemistry/water_structure.png

The structure of a molecule is defined by the symbols and the nuclear coordinates of its constituent atoms. It can be specified using different chemical file formats. Within PennyLane, the molecular structure is defined by providing a list with the atomic symbols and a one-dimensional array with the nuclear coordinates in atomic units.

import numpy as np

symbols = ["H", "O", "H"]
coordinates = np.array([[-0.0399, -0.0038, 0.0], [1.5780, 0.8540, 0.0], [2.7909, -0.5159, 0.0]])

The read_structure() function can also be used to read the molecular geometry from an external file.

from pennylane import qchem

symbols, coordinates = qchem.read_structure("quantum_chemistry/h2o.xyz")

The xyz format is supported.

Solving the Hartree-Fock equations

The molecule’s electronic Hamiltonian is commonly represented using the second-quantization formalism, which we will explore in more detail in the next section. To that aim, a basis of single-particle states needs to be chosen. In quantum chemistry these states are the molecular orbitals which describe the wave function of a single electron in the molecule.

Molecular orbitals are typically represented as a linear combination of atomic orbitals. The expansion coefficients in the atomic basis are calculated using the Hartree-Fock (HF) method. In the HF approximation, each electron in the molecule is treated as an independent particle that moves under the influence of the Coulomb potential due to the nuclei, and a mean field generated by all other electrons 3. The optimized coefficients are precisely what we need to build the second-quantized Hamiltonian.

PennyLane provides a differentiable Hartree-Fock solver and the functionality to construct a fully-differentiable molecular Hamiltonian.

Building the Hamiltonian

In the second quantization formalism, the electronic wave function of the molecule is represented in the occupation number basis. For \(M\) spin molecular orbitals, the elements of this basis are labelled as \(\vert n_0, n_1, \dots, n_{M-1} \rangle,\) where \(n_i = 0,1\) indicates the occupation of each orbital. In this representation, the electronic Hamiltonian is given by

\[H = \sum_{p,q} h_{pq} c_p^\dagger c_q + \frac{1}{2} \sum_{p,q,r,s} h_{pqrs} c_p^\dagger c_q^\dagger c_r c_s,\]

where \(c^\dagger\) and \(c\) are the electron creation and annihilation operators, respectively, and the coefficients \(h_{pq}\) and \(h_{pqrs}\) denote the one- and two-electron Coulomb integrals 4 evaluated using the Hartree-Fock orbitals.

We can use the states of \(M\) qubits to encode any element of the occupation number basis

\[\vert n_0, n_1, \dots, n_{M-1} \rangle \rightarrow \vert q_0 q_1 \cdots q_{M-1} \rangle.\]

This implies that we need to map the fermionic operators onto operators that act on qubits. This can be done by using the Jordan-Wigner transformation 5 which allows us to decompose the fermionic Hamiltonian into a linear combination of the tensor product of Pauli operators

\[H = \sum_j C_j \otimes_i \sigma_i^{(j)},\]

where \(C_j\) is a scalar coefficient and \(\sigma_i\) represents an element of the Pauli group \(\{ I, X, Y, Z \}.\)

In PennyLane we have the molecular_hamiltonian() function which encapsulates all the steps explained above. It simplifies the process of building the electronic Hamiltonian to a single line of code. We just need to input the molecule, as shown below:

molecule = qchem.Molecule(symbols, coordinates)
H, qubits = qchem.molecular_hamiltonian(molecule)
print("Number of qubits: {:}".format(qubits))
print("Qubit Hamiltonian")
print(H)

Number of qubits: 14
Qubit Hamiltonian
-46.46390691340743 * I([0, 1, 2, 3, 4, 5, 6, 7, 8, 9, 10, 11, 12, 13]) + 12.41263071443688 * Z(0) + -0.1250703688397044 * (Y(0) @ Z(1) @ Y(2)) + -0.1250703688397044 * (X(0) @ Z(1) @ X(2)) + -3.2020719246986146e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4)) + -3.2020719246986146e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4)) + 0.0427432600629203 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + 0.0427432600629203 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + -0.0716505625004305 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.0716505625004305 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -1.3986653447102222e-05 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -1.3986653447102222e-05 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.6538938305463717 * Z(2) + 0.23671071740410074 * (Z(0) @ Z(2)) + -3.886639484514147e-06 * (Y(2) @ Z(3) @ Y(4)) + -3.886639484514147e-06 * (X(2) @ Z(3) @ X(4)) + -8.336695435061184e-07 * (Z(0) @ Y(2) @ Z(3) @ Y(4)) + -8.336695435061184e-07 * (Z(0) @ X(2) @ Z(3) @ X(4)) + 0.12133242248344567 * (Y(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + 0.12133242248344567 * (X(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + 0.027114878580393256 * (Z(0) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + 0.027114878580393256 * (Z(0) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + -0.28164335753398967 * (Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.28164335753398967 * (X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -0.06752398179962302 * (Z(0) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.06752398179962302 * (Z(0) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -5.775872052630413e-05 * (Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -5.775872052630413e-05 * (X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -1.4016916321650758e-05 * (Z(0) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -1.4016916321650758e-05 * (Z(0) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.203439339131166 * Z(4) + 0.19661749959726188 * (Z(0) @ Z(4)) + 1.2260276819707572e-05 * (Y(4) @ Z(5) @ Y(6)) + 1.2260276819707572e-05 * (X(4) @ Z(5) @ X(6)) + 3.099296617465047e-06 * (Z(0) @ Y(4) @ Z(5) @ Y(6)) + 3.099296617465047e-06 * (Z(0) @ X(4) @ Z(5) @ X(6)) + -6.631261889153466e-05 * (Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -6.631261889153466e-05 * (X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -1.5316614006549205e-05 * (Z(0) @ Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -1.5316614006549205e-05 * (Z(0) @ X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + 0.36937137554444677 * (Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 0.36937137554444677 * (X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 0.08684736029515176 * (Z(0) @ Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 0.08684736029515176 * (Z(0) @ X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.3096876618630091 * Z(6) + 0.24164696831747648 * (Z(0) @ Z(6)) + -0.22847946311059097 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.22847946311059097 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -0.05608449432299921 * (Z(0) @ Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.05608449432299921 * (Z(0) @ X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -2.5950813350578864e-05 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -2.5950813350578864e-05 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -6.652106301502696e-06 * (Z(0) @ Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -6.652106301502696e-06 * (Z(0) @ X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.3693525711702206 * Z(8) + 0.2723251845037445 * (Z(0) @ Z(8)) + 0.782965207048719 * Z(10) + 0.1929970026986182 * (Z(0) @ Z(10)) + 1.0722748541094455e-05 * (Y(10) @ Z(11) @ Y(12)) + 1.0722748541094455e-05 * (X(10) @ Z(11) @ X(12)) + 2.1777330117672856e-06 * (Z(0) @ Y(10) @ Z(11) @ Y(12)) + 2.1777330117672856e-06 * (Z(0) @ X(10) @ Z(11) @ X(12)) + 0.8084591005185926 * Z(12) + 0.2110268123428544 * (Z(0) @ Z(12)) + 12.412630714436878 * Z(1) + 1.1861764484127464 * (Z(0) @ Z(1)) + -0.10433061485305181 * (Y(0) @ Y(2)) + -0.10433061485305181 * (X(0) @ X(2)) + -3.1173663779730197e-06 * (Y(0) @ Z(2) @ Z(3) @ Y(4)) + -3.1173663779730197e-06 * (X(0) @ Z(2) @ Z(3) @ X(4)) + 0.04587942403068262 * (Y(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + 0.04587942403068262 * (X(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + -0.05859215179546557 * (Y(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.05859215179546557 * (X(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -1.1462850890543263e-05 * (Y(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -1.1462850890543263e-05 * (X(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -0.12507036883970438 * (Y(1) @ Z(2) @ Y(3)) + -0.10433061485305181 * (Z(0) @ Y(1) @ Z(2) @ Y(3)) + -0.12507036883970438 * (X(1) @ Z(2) @ X(3)) + -0.10433061485305181 * (Z(0) @ X(1) @ Z(2) @ X(3)) + 0.014583638327003516 * (Y(0) @ X(1) @ X(2) @ Y(3)) + -0.014583638327003516 * (Y(0) @ Y(1) @ X(2) @ X(3)) + -0.014583638327003516 * (X(0) @ X(1) @ Y(2) @ Y(3)) + 0.014583638327003516 * (X(0) @ Y(1) @ Y(2) @ X(3)) + -3.5706354730830834e-07 * (Y(0) @ X(1) @ X(3) @ Y(4)) + -3.5706354730830834e-07 * (Y(0) @ Y(1) @ Y(3) @ Y(4)) + -3.5706354730830834e-07 * (X(0) @ X(1) @ X(3) @ X(4)) + -3.5706354730830834e-07 * (X(0) @ Y(1) @ Y(3) @ X(4)) + 0.005652607315220227 * (Y(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Y(6)) + 0.005652607315220227 * (Y(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Y(6)) + 0.005652607315220227 * (X(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ X(6)) + 0.005652607315220227 * (X(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ X(6)) + -0.008826387567791973 * (Y(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.008826387567791973 * (Y(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.008826387567791973 * (X(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -0.008826387567791973 * (X(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -1.7924638153683944e-06 * (Y(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -1.7924638153683944e-06 * (Y(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -1.7924638153683944e-06 * (X(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -1.7924638153683944e-06 * (X(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -3.2020719246986163e-06 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5)) + -3.11736637797302e-06 * (Z(0) @ Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5)) + -3.2020719246986163e-06 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5)) + -3.11736637797302e-06 * (Z(0) @ X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5)) + 3.5706354730830834e-07 * (Y(0) @ X(1) @ X(2) @ Z(3) @ Z(4) @ Y(5)) + -3.5706354730830834e-07 * (Y(0) @ Y(1) @ X(2) @ Z(3) @ Z(4) @ X(5)) + -3.5706354730830834e-07 * (X(0) @ X(1) @ Y(2) @ Z(3) @ Z(4) @ Y(5)) + 3.5706354730830834e-07 * (X(0) @ Y(1) @ Y(2) @ Z(3) @ Z(4) @ X(5)) + 0.0027458273154238448 * (Y(0) @ X(1) @ X(4) @ Y(5)) + -0.0027458273154238448 * (Y(0) @ Y(1) @ X(4) @ X(5)) + -0.0027458273154238448 * (X(0) @ X(1) @ Y(4) @ Y(5)) + 0.0027458273154238448 * (X(0) @ Y(1) @ Y(4) @ X(5)) + 2.447264796890413e-07 * (Y(0) @ X(1) @ X(5) @ Y(6)) + 2.447264796890413e-07 * (Y(0) @ Y(1) @ Y(5) @ Y(6)) + 2.447264796890413e-07 * (X(0) @ X(1) @ X(5) @ X(6)) + 2.447264796890413e-07 * (X(0) @ Y(1) @ Y(5) @ X(6)) + -7.867608556991863e-07 * (Y(0) @ X(1) @ X(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -7.867608556991863e-07 * (Y(0) @ Y(1) @ Y(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) 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X(10) @ Y(11)) + -0.01782501193262924 * (Y(6) @ Y(7) @ X(10) @ X(11)) + -0.01782501193262924 * (X(6) @ X(7) @ Y(10) @ Y(11)) + 0.01782501193262924 * (X(6) @ Y(7) @ Y(10) @ X(11)) + 1.0357924731874742e-06 * (Y(6) @ X(7) @ X(11) @ Y(12)) + 1.0357924731874742e-06 * (Y(6) @ Y(7) @ Y(11) @ Y(12)) + 1.0357924731874742e-06 * (X(6) @ X(7) @ X(11) @ X(12)) + 1.0357924731874742e-06 * (X(6) @ Y(7) @ Y(11) @ X(12)) + -3.769583576588675e-06 * (Z(6) @ Y(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Z(12) @ Y(13)) + -3.769583576588675e-06 * (Z(6) @ X(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Z(12) @ X(13)) + -1.0357924731874742e-06 * (Y(6) @ X(7) @ X(10) @ Z(11) @ Z(12) @ Y(13)) + 1.0357924731874742e-06 * (Y(6) @ Y(7) @ X(10) @ Z(11) @ Z(12) @ X(13)) + 1.0357924731874742e-06 * (X(6) @ X(7) @ Y(10) @ Z(11) @ Z(12) @ Y(13)) + -1.0357924731874742e-06 * (X(6) @ Y(7) @ Y(10) @ Z(11) @ Z(12) @ X(13)) + 0.01736605326462418 * (Y(6) @ X(7) @ X(12) @ Y(13)) + -0.01736605326462418 * (Y(6) @ Y(7) @ X(12) @ X(13)) + 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Z(12) @ Y(13) @ Z(7) @ Y(8)) + -3.32803963883771e-07 * (Y(6) @ X(9) @ Z(10) @ Z(11) @ Z(12) @ X(13) @ Z(7) @ Y(8)) + -3.32803963883771e-07 * (X(6) @ Y(9) @ Z(10) @ Z(11) @ Z(12) @ Y(13) @ Z(7) @ X(8)) + -3.32803963883771e-07 * (X(6) @ X(9) @ Z(10) @ Z(11) @ Z(12) @ X(13) @ Z(7) @ X(8)) + -3.211187414810593e-06 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(11) @ Y(12)) + -3.211187414810593e-06 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(11) @ X(12)) + -0.025104907970070967 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10) @ Z(12)) + -0.025104907970070967 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10) @ Z(12)) + 0.13734942210159606 * (Z(6) @ Z(11)) + -0.011307208030056025 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10) @ Z(11)) + -0.011307208030056025 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10) @ Z(11)) + -6.5242044662320794e-06 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Y(12)) + -6.5242044662320794e-06 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ X(12)) + 2.890929956611034e-06 * (Z(6) @ Y(11) @ Z(12) @ Y(13)) + 2.890929956611034e-06 * (Z(6) @ X(11) @ Z(12) @ X(13)) + 3.3130170514284255e-06 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10) @ Y(11) @ Z(12) @ Y(13)) + 3.3130170514284255e-06 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10) @ X(11) @ Z(12) @ X(13)) + 3.3130170514284255e-06 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10) @ Y(11) @ Z(12) @ Y(13)) + 3.3130170514284255e-06 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10) @ X(11) @ Z(12) @ X(13)) + -0.014564473640807688 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ X(11) @ X(12) @ Y(13)) + 0.014564473640807688 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11) @ X(12) @ X(13)) + 0.014564473640807688 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ X(11) @ Y(12) @ Y(13)) + -0.014564473640807688 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11) @ Y(12) @ X(13)) + 0.15138342699120916 * (Z(6) @ Z(13)) + -0.010540434329263278 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10) @ Z(13)) + -0.010540434329263278 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10) @ Z(13)) + 4.183808768020922e-06 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12) @ Z(13)) + 4.183808768020922e-06 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12) @ Z(13)) + 0.16756669356176987 * (Z(7) @ Z(9)) + 0.11952441016896681 * (Z(7) @ Z(11)) + 1.8551374834276796e-06 * (Z(7) @ Y(11) @ Z(12) @ Y(13)) + 1.8551374834276796e-06 * (Z(7) @ X(11) @ Z(12) @ X(13)) + 0.13401737372658498 * (Z(7) @ Z(13)) + 0.18144009362940672 * (Z(7) @ Z(8)) + -0.029812299601151393 * (Y(7) @ Z(9) @ Z(10) @ Y(11)) + -0.029812299601151393 * (X(7) @ Z(9) @ Z(10) @ X(11)) + -3.2774382537834046e-06 * (Y(7) @ Z(9) @ Z(10) @ Z(11) @ Z(12) @ Y(13)) + -3.2774382537834046e-06 * (X(7) @ Z(9) @ Z(10) @ Z(11) @ Z(12) @ X(13)) + -0.0002922256724522417 * (Y(7) @ X(8) @ X(9) @ Y(10)) + 0.0002922256724522417 * (Y(7) @ Y(8) @ X(9) @ X(10)) + 0.0002922256724522417 * (X(7) @ X(8) @ Y(9) @ Y(10)) + -0.0002922256724522417 * (X(7) @ Y(8) @ Y(9) @ X(10)) + -3.32803963883771e-07 * (Y(7) @ X(8) @ X(9) @ Z(10) @ Z(11) @ Y(12)) + 3.32803963883771e-07 * (Y(7) @ Y(8) @ X(9) @ Z(10) @ Z(11) @ X(12)) + 3.32803963883771e-07 * (X(7) @ X(8) @ Y(9) @ Z(10) @ Z(11) @ Y(12)) + -3.32803963883771e-07 * (X(7) @ Y(8) @ Y(9) @ Z(10) @ Z(11) @ X(12)) + -0.030104525273603633 * (Y(7) @ Z(8) @ Z(10) @ Y(11)) + -0.030104525273603633 * (X(7) @ Z(8) @ Z(10) @ X(11)) + -3.6102422176671756e-06 * (Y(7) @ Z(8) @ Z(10) @ Z(11) @ Z(12) @ Y(13)) + -3.6102422176671756e-06 * (X(7) @ Z(8) @ Z(10) @ Z(11) @ Z(12) @ X(13)) + 0.13734942210159606 * (Z(7) @ Z(10)) + -0.011307208030056025 * (Y(7) @ Z(8) @ Z(9) @ Y(11)) + -0.011307208030056025 * (X(7) @ Z(8) @ Z(9) @ X(11)) + -6.5242044662320794e-06 * (Y(7) @ Z(8) @ Z(9) @ Z(11) @ Z(12) @ Y(13)) + -6.5242044662320794e-06 * (X(7) @ Z(8) @ Z(9) @ Z(11) @ Z(12) @ X(13)) + 2.890929956611034e-06 * (Z(7) @ Y(10) @ Z(11) @ Y(12)) + 2.890929956611034e-06 * (Z(7) @ X(10) @ Z(11) @ X(12)) + 3.3130170514284255e-06 * (Y(7) @ Z(8) @ Z(9) @ X(10) @ X(11) @ Y(12)) + -3.3130170514284255e-06 * (Y(7) @ Z(8) @ Z(9) @ Y(10) @ X(11) @ X(12)) + -3.3130170514284255e-06 * (X(7) @ Z(8) @ Z(9) @ X(10) @ Y(11) @ Y(12)) + 3.3130170514284255e-06 * (X(7) @ Z(8) @ Z(9) @ Y(10) @ Y(11) @ X(12)) + 0.01456447364080769 * (Y(7) @ Z(8) @ Z(9) @ X(10) @ X(12) @ Y(13)) + 0.01456447364080769 * (Y(7) @ Z(8) @ Z(9) @ Y(10) @ Y(12) @ Y(13)) + 0.01456447364080769 * (X(7) @ Z(8) @ Z(9) @ X(10) @ X(12) @ X(13)) + 0.01456447364080769 * (X(7) @ Z(8) @ Z(9) @ Y(10) @ Y(12) @ X(13)) + -3.211187414810593e-06 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Z(12) @ Y(13)) + -3.211187414810593e-06 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ Z(12) @ X(13)) + -0.025104907970070967 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11) @ Z(13)) + -0.025104907970070967 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ X(11) @ Z(13)) + 0.15138342699120916 * (Z(7) @ Z(12)) + -0.010540434329263278 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11) @ Z(12)) + -0.010540434329263278 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ X(11) @ Z(12)) + 4.183808768020922e-06 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(13)) + 4.183808768020922e-06 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(13)) + 0.137668591336212 * (Z(8) @ Z(10)) + 1.5973397403137813e-06 * (Z(8) @ Y(10) @ Z(11) @ Y(12)) + 1.5973397403137813e-06 * (Z(8) @ X(10) @ Z(11) @ X(12)) + 0.14973497005438616 * (Z(8) @ Z(12)) + 0.2200397724028209 * (Z(8) @ Z(9)) + 0.009560716496448234 * (Y(8) @ X(9) @ X(10) @ Y(11)) + -0.009560716496448234 * (Y(8) @ Y(9) @ X(10) @ X(11)) + -0.009560716496448234 * (X(8) @ X(9) @ Y(10) @ Y(11)) + 0.009560716496448234 * (X(8) @ Y(9) @ Y(10) @ X(11)) + -6.628427195201582e-07 * (Y(8) @ X(9) @ X(11) @ Y(12)) + -6.628427195201582e-07 * (Y(8) @ Y(9) @ Y(11) @ Y(12)) + -6.628427195201582e-07 * (X(8) @ X(9) @ X(11) @ X(12)) + -6.628427195201582e-07 * (X(8) @ Y(9) @ Y(11) @ X(12)) + 6.628427195201582e-07 * (Y(8) @ X(9) @ X(10) @ Z(11) @ Z(12) @ Y(13)) + -6.628427195201582e-07 * (Y(8) @ Y(9) @ X(10) @ Z(11) @ Z(12) @ X(13)) + -6.628427195201582e-07 * (X(8) @ X(9) @ Y(10) @ Z(11) @ Z(12) @ Y(13)) + 6.628427195201582e-07 * (X(8) @ Y(9) @ Y(10) @ Z(11) @ Z(12) @ X(13)) + 0.006087836804235006 * (Y(8) @ X(9) @ X(12) @ Y(13)) + -0.006087836804235006 * (Y(8) @ Y(9) @ X(12) @ X(13)) + -0.006087836804235006 * (X(8) @ X(9) @ Y(12) @ Y(13)) + 0.006087836804235006 * (X(8) @ Y(9) @ Y(12) @ X(13)) + 0.14722930783266025 * (Z(8) @ Z(11)) + 9.344970207936232e-07 * (Z(8) @ Y(11) @ Z(12) @ Y(13)) + 9.344970207936232e-07 * (Z(8) @ X(11) @ Z(12) @ X(13)) + 0.15582280685862115 * (Z(8) @ Z(13)) + 0.137668591336212 * (Z(9) @ Z(11)) + 1.5973397403137813e-06 * (Z(9) @ Y(11) @ Z(12) @ Y(13)) + 1.5973397403137813e-06 * (Z(9) @ X(11) @ Z(12) @ X(13)) + 0.14973497005438616 * (Z(9) @ Z(13)) + 0.14722930783266025 * (Z(9) @ Z(10)) + 9.344970207936232e-07 * (Z(9) @ Y(10) @ Z(11) @ Y(12)) + 9.344970207936232e-07 * (Z(9) @ X(10) @ Z(11) @ X(12)) + 0.15582280685862115 * (Z(9) @ Z(12)) + 0.1127038185912413 * (Z(10) @ Z(12)) + 0.14926347060044898 * (Z(10) @ Z(11)) + 8.194104947113062e-06 * (Y(10) @ Y(12)) + 8.194104947113062e-06 * (X(10) @ X(12)) + 8.194104947113062e-06 * (Z(10) @ Y(11) @ Z(12) @ Y(13)) + 8.194104947113062e-06 * (Z(10) @ X(11) @ Z(12) @ X(13)) + 0.028685217310290168 * (Y(10) @ X(11) @ X(12) @ Y(13)) + -0.028685217310290168 * (Y(10) @ Y(11) @ X(12) @ X(13)) + -0.028685217310290168 * (X(10) @ X(11) @ Y(12) @ Y(13)) + 0.028685217310290168 * (X(10) @ Y(11) @ Y(12) @ X(13)) + 0.14138903590153146 * (Z(10) @ Z(13)) + -7.954224535706989e-06 * (Y(10) @ Z(11) @ Y(12) @ Z(13)) + -7.954224535706989e-06 * (X(10) @ Z(11) @ X(12) @ Z(13)) + 0.1127038185912413 * (Z(11) @ Z(13)) + 0.14138903590153146 * (Z(11) @ Z(12)) + -7.954224535706989e-06 * (Y(11) @ Y(13)) + -7.954224535706989e-06 * (X(11) @ X(13)) + 0.15435760065309656 * (Z(12) @ Z(13))

Advanced features

The Molecule object allows us to define additional keyword arguments to solve the Hartree-Fock equations of more complicated systems. The net charge of the molecule may be specified to simulate positively or negatively charged molecules. For a neutral system we choose

charge = 0

We can also specify the spin multiplicity. For the water molecule, which contains ten electrons, the Slater determinant resulting from occupying the five lowest-energy orbitals with two paired electrons per orbital has spin multiplicity one. Alternatively, if we define an occupation where the first four orbitals are doubly occupied and the next two are singly occupied by unpaired electrons, the HF state will have multiplicity three.


demos/_static/demonstration_assets/quantum_chemistry/hf_references.png

For the neutral water molecule we have,

multiplicity = 1

As mentioned above, molecular orbitals are represented as a linear combination of atomic orbitals which are typically modeled as Gaussian-type orbitals. We can specify different types of Gaussian atomic bases. In this example we choose a minimal basis set.

basis_set = "sto-3g"

PennyLane also allows us to define an active space 6 to perform quantum simulations with a reduced number of qubits. This is done by classifying the molecular orbitals as core, active, and external orbitals:

  • Core orbitals are always occupied by two electrons.

  • Active orbitals can be occupied by zero, one, or two electrons.

  • The external orbitals are never occupied.

Within this approximation, a certain number of active electrons are allowed to populate a finite set of active orbitals.

demos/_static/demonstration_assets/quantum_chemistry/sketch_active_space.png

Note

The number of active spin-orbitals determines the number of qubits required to perform the quantum simulations.

For the water molecule in a minimal basis set we have a total of ten electrons and seven molecular orbitals. In this example we define a symmetric active space with four electrons and four active orbitals using the active_space() function:

electrons = 10
orbitals = 7
core, active = qchem.active_space(electrons, orbitals, active_electrons=4, active_orbitals=4)

Viewing the results:

print("List of core orbitals: {:}".format(core))
print("List of active orbitals: {:}".format(active))
print("Number of qubits: {:}".format(2 * len(active)))

List of core orbitals: [0, 1, 2]
List of active orbitals: [3, 4, 5, 6]
Number of qubits: 8

Finally, we use the molecular_hamiltonian() function to build the resulting Hamiltonian of the water molecule:

molecule = qchem.Molecule(
    symbols,
    coordinates,
    charge=charge,
    mult=multiplicity,
    basis_name=basis_set
)

H, qubits = qchem.molecular_hamiltonian(
    molecule,
    active_electrons=4,
    active_orbitals=4,
)

print("Number of qubits required to perform quantum simulations: {:}".format(qubits))
print("Hamiltonian of the water molecule")
print(H)

Number of qubits required to perform quantum simulations: 8
Hamiltonian of the water molecule
-73.13873149595426 * I([0, 1, 2, 3, 4, 5, 6, 7]) + 0.227573288144638 * Z(0) + -0.04375171612137361 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4)) + -0.04375171612137361 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4)) + -5.105681029587138e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + -5.105681029587138e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + 0.17419986612111382 * Z(2) + 0.16756669356176987 * (Z(0) @ Z(2)) + -0.1596144358374325 * Z(4) + 0.11952441016896681 * (Z(0) @ Z(4)) + 7.038023727338103e-06 * (Y(4) @ Z(5) @ Y(6)) + 7.038023727338103e-06 * (X(4) @ Z(5) @ X(6)) + 1.8551374834276796e-06 * (Z(0) @ Y(4) @ Z(5) @ Y(6)) + 1.8551374834276796e-06 * (Z(0) @ X(4) @ Z(5) @ X(6)) + -0.1806675750702108 * Z(6) + 0.13401737372658498 * (Z(0) @ Z(6)) + 0.2275732881446381 * Z(1) + 0.19392574334986945 * (Z(0) @ Z(1)) + -0.030787440718630918 * (Y(0) @ Z(2) @ Z(3) @ Y(4)) + -0.030787440718630918 * (X(0) @ Z(2) @ Z(3) @ X(4)) + -3.769583576588675e-06 * (Y(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + -3.769583576588675e-06 * (X(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + 0.013873400067636855 * (Y(0) @ X(1) @ X(2) @ Y(3)) + -0.013873400067636855 * (Y(0) @ Y(1) @ X(2) @ X(3)) + -0.013873400067636855 * (X(0) @ X(1) @ Y(2) @ Y(3)) + 0.013873400067636855 * (X(0) @ Y(1) @ Y(2) @ X(3)) + -0.043751716121373595 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5)) + -0.030787440718630918 * (Z(0) @ Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5)) + -0.043751716121373595 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5)) + -0.030787440718630918 * (Z(0) @ X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5)) + 0.01782501193262924 * (Y(0) @ X(1) @ X(4) @ Y(5)) + -0.01782501193262924 * (Y(0) @ Y(1) @ X(4) @ X(5)) + -0.01782501193262924 * (X(0) @ X(1) @ Y(4) @ Y(5)) + 0.01782501193262924 * (X(0) @ Y(1) @ Y(4) @ X(5)) + 1.0357924731874742e-06 * (Y(0) @ X(1) @ X(5) @ Y(6)) + 1.0357924731874742e-06 * (Y(0) @ Y(1) @ Y(5) @ Y(6)) + 1.0357924731874742e-06 * (X(0) @ X(1) @ X(5) @ X(6)) + 1.0357924731874742e-06 * (X(0) @ Y(1) @ Y(5) @ X(6)) + -5.105681029587138e-06 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + -3.769583576588675e-06 * (Z(0) @ Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + -5.105681029587138e-06 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + -3.769583576588675e-06 * (Z(0) @ X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + -1.0357924731874742e-06 * (Y(0) @ X(1) @ X(4) @ Z(5) @ Z(6) @ Y(7)) + 1.0357924731874742e-06 * (Y(0) @ Y(1) @ X(4) @ Z(5) @ Z(6) @ X(7)) + 1.0357924731874742e-06 * (X(0) @ X(1) @ Y(4) @ Z(5) @ Z(6) @ Y(7)) + -1.0357924731874742e-06 * (X(0) @ Y(1) @ Y(4) @ Z(5) @ Z(6) @ X(7)) + 0.01736605326462418 * (Y(0) @ X(1) @ X(6) @ Y(7)) + -0.01736605326462418 * (Y(0) @ Y(1) @ X(6) @ X(7)) + -0.01736605326462418 * (X(0) @ X(1) @ Y(6) @ Y(7)) + 0.01736605326462418 * (X(0) @ Y(1) @ Y(6) @ X(7)) + -0.030104525273603633 * (Y(0) @ Z(1) @ Z(3) @ Y(4)) + -0.030104525273603633 * (X(0) @ Z(1) @ Z(3) @ X(4)) + -3.6102422176671756e-06 * (Y(0) @ Z(1) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + -3.6102422176671756e-06 * (X(0) @ Z(1) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + 0.17419986612111385 * Z(3) + 0.18144009362940672 * (Z(0) @ Z(3)) + -0.029812299601151393 * (Y(0) @ Z(1) @ Z(2) @ Y(4)) + -0.029812299601151393 * (X(0) @ Z(1) @ Z(2) @ X(4)) + -3.2774382537834046e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(4) @ Z(5) @ Y(6)) + -3.2774382537834046e-06 * (X(0) @ Z(1) @ Z(2) @ Z(4) @ Z(5) @ X(6)) + -0.0002922256724522417 * (Y(0) @ Y(3) @ Z(4) @ Y(5) @ Z(1) @ Y(2)) + -0.0002922256724522417 * (Y(0) @ X(3) @ Z(4) @ X(5) @ Z(1) @ Y(2)) + -0.0002922256724522417 * (X(0) @ Y(3) @ Z(4) @ Y(5) @ Z(1) @ X(2)) + -0.0002922256724522417 * (X(0) @ X(3) @ Z(4) @ X(5) @ Z(1) @ X(2)) + -3.32803963883771e-07 * (Y(0) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7) @ Z(1) @ Y(2)) + -3.32803963883771e-07 * (Y(0) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ X(7) @ Z(1) @ Y(2)) + -3.32803963883771e-07 * (X(0) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7) @ Z(1) @ X(2)) + -3.32803963883771e-07 * (X(0) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ X(7) @ Z(1) @ X(2)) + -3.211187414810593e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(5) @ Y(6)) + -3.211187414810593e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(5) @ X(6)) + -0.025104907970070967 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4) @ Z(6)) + -0.025104907970070967 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4) @ Z(6)) + -0.1596144358374324 * Z(5) + 0.13734942210159606 * (Z(0) @ Z(5)) + -0.011307208030056025 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4) @ Z(5)) + -0.011307208030056025 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4) @ Z(5)) + -6.5242044662320794e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Y(6)) + -6.5242044662320794e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ X(6)) + 7.038023727338103e-06 * (Y(5) @ Z(6) @ Y(7)) + 2.890929956611034e-06 * (Z(0) @ Y(5) @ Z(6) @ Y(7)) + 7.038023727338103e-06 * (X(5) @ Z(6) @ X(7)) + 2.890929956611034e-06 * (Z(0) @ X(5) @ Z(6) @ X(7)) + 3.3130170514284255e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4) @ Y(5) @ Z(6) @ Y(7)) + 3.3130170514284255e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4) @ X(5) @ Z(6) @ X(7)) + 3.3130170514284255e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4) @ Y(5) @ Z(6) @ Y(7)) + 3.3130170514284255e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4) @ X(5) @ Z(6) @ X(7)) + -0.014564473640807688 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ X(5) @ X(6) @ Y(7)) + 0.014564473640807688 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5) @ X(6) @ X(7)) + 0.014564473640807688 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ X(5) @ Y(6) @ Y(7)) + -0.014564473640807688 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5) @ Y(6) @ X(7)) + -0.18066757507021058 * Z(7) + 0.15138342699120916 * (Z(0) @ Z(7)) + -0.010540434329263278 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4) @ Z(7)) + -0.010540434329263278 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4) @ Z(7)) + 4.183808768020922e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6) @ Z(7)) + 4.183808768020922e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(6) @ Z(7)) + 0.16756669356176987 * (Z(1) @ Z(3)) + 0.11952441016896681 * (Z(1) @ Z(5)) + 1.8551374834276796e-06 * (Z(1) @ Y(5) @ Z(6) @ Y(7)) + 1.8551374834276796e-06 * (Z(1) @ X(5) @ Z(6) @ X(7)) + 0.13401737372658498 * (Z(1) @ Z(7)) + 0.18144009362940672 * (Z(1) @ Z(2)) + -0.029812299601151393 * (Y(1) @ Z(3) @ Z(4) @ Y(5)) + -0.029812299601151393 * (X(1) @ Z(3) @ Z(4) @ X(5)) + -3.2774382537834046e-06 * (Y(1) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + -3.2774382537834046e-06 * (X(1) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + -0.0002922256724522417 * (Y(1) @ X(2) @ X(3) @ Y(4)) + 0.0002922256724522417 * (Y(1) @ Y(2) @ X(3) @ X(4)) + 0.0002922256724522417 * (X(1) @ X(2) @ Y(3) @ Y(4)) + -0.0002922256724522417 * (X(1) @ Y(2) @ Y(3) @ X(4)) + -3.32803963883771e-07 * (Y(1) @ X(2) @ X(3) @ Z(4) @ Z(5) @ Y(6)) + 3.32803963883771e-07 * (Y(1) @ Y(2) @ X(3) @ Z(4) @ Z(5) @ X(6)) + 3.32803963883771e-07 * (X(1) @ X(2) @ Y(3) @ Z(4) @ Z(5) @ Y(6)) + -3.32803963883771e-07 * (X(1) @ Y(2) @ Y(3) @ Z(4) @ Z(5) @ X(6)) + -0.030104525273603633 * (Y(1) @ Z(2) @ Z(4) @ Y(5)) + -0.030104525273603633 * (X(1) @ Z(2) @ Z(4) @ X(5)) + -3.6102422176671756e-06 * (Y(1) @ Z(2) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + -3.6102422176671756e-06 * (X(1) @ Z(2) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + 0.13734942210159606 * (Z(1) @ Z(4)) + -0.011307208030056025 * (Y(1) @ Z(2) @ Z(3) @ Y(5)) + -0.011307208030056025 * (X(1) @ Z(2) @ Z(3) @ X(5)) + -6.5242044662320794e-06 * (Y(1) @ Z(2) @ Z(3) @ Z(5) @ Z(6) @ Y(7)) + -6.5242044662320794e-06 * (X(1) @ Z(2) @ Z(3) @ Z(5) @ Z(6) @ X(7)) + 2.890929956611034e-06 * (Z(1) @ Y(4) @ Z(5) @ Y(6)) + 2.890929956611034e-06 * (Z(1) @ X(4) @ Z(5) @ X(6)) + 3.3130170514284255e-06 * (Y(1) @ Z(2) @ Z(3) @ X(4) @ X(5) @ Y(6)) + -3.3130170514284255e-06 * (Y(1) @ Z(2) @ Z(3) @ Y(4) @ X(5) @ X(6)) + -3.3130170514284255e-06 * (X(1) @ Z(2) @ Z(3) @ X(4) @ Y(5) @ Y(6)) + 3.3130170514284255e-06 * (X(1) @ Z(2) @ Z(3) @ Y(4) @ Y(5) @ X(6)) + 0.01456447364080769 * (Y(1) @ Z(2) @ Z(3) @ X(4) @ X(6) @ Y(7)) + 0.01456447364080769 * (Y(1) @ Z(2) @ Z(3) @ Y(4) @ Y(6) @ Y(7)) + 0.01456447364080769 * (X(1) @ Z(2) @ Z(3) @ X(4) @ X(6) @ X(7)) + 0.01456447364080769 * (X(1) @ Z(2) @ Z(3) @ Y(4) @ Y(6) @ X(7)) + -3.211187414810593e-06 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(6) @ Y(7)) + -3.211187414810593e-06 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(6) @ X(7)) + -0.025104907970070967 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5) @ Z(7)) + -0.025104907970070967 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5) @ Z(7)) + 0.15138342699120916 * (Z(1) @ Z(6)) + -0.010540434329263278 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5) @ Z(6)) + -0.010540434329263278 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5) @ Z(6)) + 4.183808768020922e-06 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(7)) + 4.183808768020922e-06 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(7)) + 0.137668591336212 * (Z(2) @ Z(4)) + 1.5973397403137813e-06 * (Z(2) @ Y(4) @ Z(5) @ Y(6)) + 1.5973397403137813e-06 * (Z(2) @ X(4) @ Z(5) @ X(6)) + 0.14973497005438616 * (Z(2) @ Z(6)) + 0.2200397724028209 * (Z(2) @ Z(3)) + 0.009560716496448234 * (Y(2) @ X(3) @ X(4) @ Y(5)) + -0.009560716496448234 * (Y(2) @ Y(3) @ X(4) @ X(5)) + -0.009560716496448234 * (X(2) @ X(3) @ Y(4) @ Y(5)) + 0.009560716496448234 * (X(2) @ Y(3) @ Y(4) @ X(5)) + -6.628427195201582e-07 * (Y(2) @ X(3) @ X(5) @ Y(6)) + -6.628427195201582e-07 * (Y(2) @ Y(3) @ Y(5) @ Y(6)) + -6.628427195201582e-07 * (X(2) @ X(3) @ X(5) @ X(6)) + -6.628427195201582e-07 * (X(2) @ Y(3) @ Y(5) @ X(6)) + 6.628427195201582e-07 * (Y(2) @ X(3) @ X(4) @ Z(5) @ Z(6) @ Y(7)) + -6.628427195201582e-07 * (Y(2) @ Y(3) @ X(4) @ Z(5) @ Z(6) @ X(7)) + -6.628427195201582e-07 * (X(2) @ X(3) @ Y(4) @ Z(5) @ Z(6) @ Y(7)) + 6.628427195201582e-07 * (X(2) @ Y(3) @ Y(4) @ Z(5) @ Z(6) @ X(7)) + 0.006087836804235006 * (Y(2) @ X(3) @ X(6) @ Y(7)) + -0.006087836804235006 * (Y(2) @ Y(3) @ X(6) @ X(7)) + -0.006087836804235006 * (X(2) @ X(3) @ Y(6) @ Y(7)) + 0.006087836804235006 * (X(2) @ Y(3) @ Y(6) @ X(7)) + 0.14722930783266025 * (Z(2) @ Z(5)) + 9.344970207936232e-07 * (Z(2) @ Y(5) @ Z(6) @ Y(7)) + 9.344970207936232e-07 * (Z(2) @ X(5) @ Z(6) @ X(7)) + 0.15582280685862115 * (Z(2) @ Z(7)) + 0.137668591336212 * (Z(3) @ Z(5)) + 1.5973397403137813e-06 * (Z(3) @ Y(5) @ Z(6) @ Y(7)) + 1.5973397403137813e-06 * (Z(3) @ X(5) @ Z(6) @ X(7)) + 0.14973497005438616 * (Z(3) @ Z(7)) + 0.14722930783266025 * (Z(3) @ Z(4)) + 9.344970207936232e-07 * (Z(3) @ Y(4) @ Z(5) @ Y(6)) + 9.344970207936232e-07 * (Z(3) @ X(4) @ Z(5) @ X(6)) + 0.15582280685862115 * (Z(3) @ Z(6)) + 0.1127038185912413 * (Z(4) @ Z(6)) + 0.14926347060044898 * (Z(4) @ Z(5)) + 8.194104947113062e-06 * (Y(4) @ Y(6)) + 8.194104947113062e-06 * (X(4) @ X(6)) + 8.194104947113062e-06 * (Z(4) @ Y(5) @ Z(6) @ Y(7)) + 8.194104947113062e-06 * (Z(4) @ X(5) @ Z(6) @ X(7)) + 0.028685217310290168 * (Y(4) @ X(5) @ X(6) @ Y(7)) + -0.028685217310290168 * (Y(4) @ Y(5) @ X(6) @ X(7)) + -0.028685217310290168 * (X(4) @ X(5) @ Y(6) @ Y(7)) + 0.028685217310290168 * (X(4) @ Y(5) @ Y(6) @ X(7)) + 0.14138903590153146 * (Z(4) @ Z(7)) + -7.954224535706989e-06 * (Y(4) @ Z(5) @ Y(6) @ Z(7)) + -7.954224535706989e-06 * (X(4) @ Z(5) @ X(6) @ Z(7)) + 0.1127038185912413 * (Z(5) @ Z(7)) + 0.14138903590153146 * (Z(5) @ Z(6)) + -7.954224535706989e-06 * (Y(5) @ Y(7)) + -7.954224535706989e-06 * (X(5) @ X(7)) + 0.15435760065309656 * (Z(6) @ Z(7))

In this case, since we have truncated the basis of molecular orbitals, the resulting observable is an approximation of the Hamiltonian generated in the section Building the Hamiltonian.

OpenFermion-PySCF backend

The molecular_hamiltonian() function can also be used to construct the molecular Hamiltonian with a non-differentiable backend that uses the OpenFermion-PySCF plugin interfaced with the electronic structure package PySCF. This backend can be selected by setting method='pyscf' in molecular_hamiltonian():

molecule = qchem.Molecule(symbols, coordinates)
H, qubits = qchem.molecular_hamiltonian(molecule, method="pyscf")
print(H)

-46.46390678868892 * I([0, 1, 2, 3, 4, 5, 6, 7, 8, 9, 10, 11, 12, 13]) + 12.412630739844072 * Z(0) + 0.12507034393810074 * (Y(0) @ Z(1) @ Y(2)) + 0.12507034393810074 * (X(0) @ Z(1) @ X(2)) + 3.2020848466251125e-06 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Y(4)) + 3.2020848466251125e-06 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ X(4)) + 0.042743263145360075 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + 0.042743263145360075 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + 0.07165049915744277 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + 0.07165049915744277 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -1.3986724780305958e-05 * (Y(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -1.3986724780305958e-05 * (X(0) @ Z(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.653893935515875 * Z(2) + 0.23671074111846685 * (Z(0) @ Z(2)) + -3.886786107462742e-06 * (Y(2) @ Z(3) @ Y(4)) + -3.886786107462742e-06 * (X(2) @ Z(3) @ X(4)) + -8.337016091439186e-07 * (Z(0) @ Y(2) @ Z(3) @ Y(4)) + -8.337016091439186e-07 * (Z(0) @ X(2) @ Z(3) @ X(4)) + -0.1213325517643341 * (Y(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + -0.1213325517643341 * (X(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + -0.02711492993678006 * (Z(0) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + -0.02711492993678006 * (Z(0) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + -0.28164314352942227 * (Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.28164314352942227 * (X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -0.06752394393124578 * (Z(0) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.06752394393124578 * (Z(0) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + 5.775886158154977e-05 * (Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 5.775886158154977e-05 * (X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.4016952399759651e-05 * (Z(0) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 1.4016952399759651e-05 * (Z(0) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.2034396183646798 * Z(4) + 0.1966175652644544 * (Z(0) @ Z(4)) + -1.2260373754988836e-05 * (Y(4) @ Z(5) @ Y(6)) + -1.2260373754988836e-05 * (X(4) @ Z(5) @ X(6)) + -3.0993238529033096e-06 * (Z(0) @ Y(4) @ Z(5) @ Y(6)) + -3.0993238529033096e-06 * (Z(0) @ X(4) @ Z(5) @ X(6)) + -6.631253627395069e-05 * (Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -6.631253627395069e-05 * (X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -1.5316633421393652e-05 * (Z(0) @ Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -1.5316633421393652e-05 * (Z(0) @ X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -0.3693712201028116 * (Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -0.3693712201028116 * (X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -0.08684736387886986 * (Z(0) @ Y(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -0.08684736387886986 * (Z(0) @ X(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.3096872459198015 * Z(6) + 0.24164686828254567 * (Z(0) @ Z(6)) + 0.22847994339650998 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + 0.22847994339650998 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + 0.05608454758733886 * (Z(0) @ Y(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + 0.05608454758733886 * (Z(0) @ X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -2.5950691777656887e-05 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -2.5950691777656887e-05 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -6.652101384625076e-06 * (Z(0) @ Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -6.652101384625076e-06 * (Z(0) @ X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.369352563471822 * Z(8) + 0.2723251828676465 * (Z(0) @ Z(8)) + 0.7829655149718391 * Z(10) + 0.19299707694442478 * (Z(0) @ Z(10)) + -1.0722628013521976e-05 * (Y(10) @ Z(11) @ Y(12)) + -1.0722628013521976e-05 * (X(10) @ Z(11) @ X(12)) + -2.177710143047922e-06 * (Z(0) @ Y(10) @ Z(11) @ Y(12)) + -2.177710143047922e-06 * (Z(0) @ X(10) @ Z(11) @ X(12)) + 0.8084588067218648 * Z(12) + 0.2110267419134197 * (Z(0) @ Z(12)) + 12.41263073984407 * Z(1) + 1.186176369602945 * (Z(0) @ Z(1)) + 0.10433060969275462 * (Y(0) @ Y(2)) + 0.10433060969275462 * (X(0) @ X(2)) + 3.117400203840882e-06 * (Y(0) @ Z(2) @ Z(3) @ Y(4)) + 3.117400203840882e-06 * (X(0) @ Z(2) @ Z(3) @ X(4)) + 0.04587943712720554 * (Y(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Y(6)) + 0.04587943712720554 * (X(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ X(6)) + 0.05859209694947503 * (Y(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + 0.05859209694947503 * (X(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -1.146288698009414e-05 * (Y(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -1.146288698009414e-05 * (X(0) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 0.12507034393810074 * (Y(1) @ Z(2) @ Y(3)) + 0.10433060969275462 * (Z(0) @ Y(1) @ Z(2) @ Y(3)) + 0.12507034393810074 * (X(1) @ Z(2) @ X(3)) + 0.10433060969275462 * (Z(0) @ X(1) @ Z(2) @ X(3)) + 0.014583638707259587 * (Y(0) @ X(1) @ X(2) @ Y(3)) + -0.014583638707259587 * (Y(0) @ Y(1) @ X(2) @ X(3)) + -0.014583638707259587 * (X(0) @ X(1) @ Y(2) @ Y(3)) + 0.014583638707259587 * (X(0) @ Y(1) @ Y(2) @ X(3)) + -3.5706821107833565e-07 * (Y(0) @ X(1) @ X(3) @ Y(4)) + -3.5706821107833565e-07 * (Y(0) @ Y(1) @ Y(3) @ Y(4)) + -3.5706821107833565e-07 * (X(0) @ X(1) @ X(3) @ X(4)) + -3.5706821107833565e-07 * (X(0) @ Y(1) @ Y(3) @ X(4)) + -0.005652610978191098 * (Y(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Y(6)) + -0.005652610978191098 * (Y(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Y(6)) + -0.005652610978191098 * (X(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ X(6)) + -0.005652610978191098 * (X(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ X(6)) + -0.0088263806631776 * (Y(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.0088263806631776 * (Y(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -0.0088263806631776 * (X(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -0.0088263806631776 * (X(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + 1.7924690730873521e-06 * (Y(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 1.7924690730873521e-06 * (Y(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 1.7924690730873521e-06 * (X(0) @ X(1) @ X(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.7924690730873521e-06 * (X(0) @ Y(1) @ Y(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 3.2020848466251117e-06 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5)) + 3.117400203840882e-06 * (Z(0) @ Y(1) @ Z(2) @ Z(3) @ Z(4) @ Y(5)) + 3.2020848466251117e-06 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5)) + 3.117400203840882e-06 * (Z(0) @ X(1) @ Z(2) @ Z(3) @ Z(4) @ X(5)) + 3.5706821107833565e-07 * (Y(0) @ X(1) @ X(2) @ Z(3) @ Z(4) @ Y(5)) + -3.5706821107833565e-07 * (Y(0) @ Y(1) @ X(2) @ Z(3) @ Z(4) @ X(5)) + -3.5706821107833565e-07 * (X(0) @ X(1) @ Y(2) @ Z(3) @ Z(4) @ Y(5)) + 3.5706821107833565e-07 * (X(0) @ Y(1) @ Y(2) @ Z(3) @ Z(4) @ X(5)) + 0.0027458302455413332 * (Y(0) @ X(1) @ X(4) @ Y(5)) + -0.0027458302455413332 * (Y(0) @ Y(1) @ X(4) @ X(5)) + -0.0027458302455413332 * (X(0) @ X(1) @ Y(4) @ Y(5)) + 0.0027458302455413332 * (X(0) @ Y(1) @ Y(4) @ X(5)) + -2.4472916981610655e-07 * (Y(0) @ X(1) @ X(5) @ Y(6)) + -2.4472916981610655e-07 * (Y(0) @ Y(1) @ Y(5) @ Y(6)) + -2.4472916981610655e-07 * (X(0) @ X(1) @ X(5) @ X(6)) + -2.4472916981610655e-07 * (X(0) @ Y(1) @ Y(5) @ X(6)) + -7.867642163434014e-07 * (Y(0) @ X(1) @ X(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -7.867642163434014e-07 * (Y(0) @ Y(1) @ Y(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Y(10)) + -7.867642163434014e-07 * (X(0) @ X(1) @ X(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -7.867642163434014e-07 * (X(0) @ Y(1) @ Y(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ X(10)) + -0.0038040641513286595 * (Y(0) @ X(1) @ X(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -0.0038040641513286595 * (Y(0) @ Y(1) @ Y(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + -0.0038040641513286595 * (X(0) @ X(1) @ X(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + -0.0038040641513286595 * (X(0) @ Y(1) @ Y(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 0.04274326314536004 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + 0.04587943712720554 * (Z(0) @ Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + 0.04274326314536004 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + 0.04587943712720554 * (Z(0) @ X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + 0.005652610978191098 * (Y(0) @ X(1) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + -0.005652610978191098 * (Y(0) @ Y(1) @ X(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + -0.005652610978191098 * (X(0) @ X(1) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Y(7)) + 0.005652610978191098 * (X(0) @ Y(1) @ Y(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ X(7)) + 2.4472916981610655e-07 * (Y(0) @ X(1) @ X(4) @ Z(5) @ Z(6) @ Y(7)) + -2.4472916981610655e-07 * (Y(0) @ Y(1) @ X(4) @ Z(5) @ Z(6) @ X(7)) + -2.4472916981610655e-07 * (X(0) @ X(1) @ Y(4) @ Z(5) @ Z(6) @ Y(7)) + 2.4472916981610655e-07 * (X(0) @ Y(1) @ Y(4) @ Z(5) @ Z(6) @ X(7)) + 0.006888201529772655 * (Y(0) @ X(1) @ X(6) @ Y(7)) + -0.006888201529772655 * (Y(0) @ Y(1) @ X(6) @ X(7)) + -0.006888201529772655 * (X(0) @ X(1) @ Y(6) @ Y(7)) + 0.006888201529772655 * (X(0) @ Y(1) @ Y(6) @ X(7)) + -7.735606930216471e-05 * (Y(0) @ X(1) @ X(7) @ Z(8) @ Z(9) @ Y(10)) + -7.735606930216471e-05 * (Y(0) @ Y(1) @ Y(7) @ Z(8) @ Z(9) @ Y(10)) + -7.735606930216471e-05 * (X(0) @ X(1) @ X(7) @ Z(8) @ Z(9) @ X(10)) + -7.735606930216471e-05 * (X(0) @ Y(1) @ Y(7) @ Z(8) @ Z(9) @ X(10)) + 1.7035584295456937e-07 * (Y(0) @ X(1) @ X(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 1.7035584295456937e-07 * (Y(0) @ Y(1) @ Y(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12)) + 1.7035584295456937e-07 * (X(0) @ X(1) @ X(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 1.7035584295456937e-07 * (X(0) @ Y(1) @ Y(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12)) + 0.006509361345963717 * (Y(0) @ X(1) @ X(8) @ Y(9)) + -0.006509361345963717 * (Y(0) @ Y(1) @ X(8) @ X(9)) + -0.006509361345963717 * (X(0) @ X(1) @ Y(8) @ Y(9)) + 0.006509361345963717 * (X(0) @ Y(1) @ Y(8) @ X(9)) + 0.07165049915744276 * (Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11)) + 0.05859209694947503 * (Z(0) @ Y(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11)) + 0.07165049915744276 * (X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ X(11)) + 0.05859209694947503 * (Z(0) @ X(1) @ Z(2) @ Z(3) @ Z(4) @ Z(5) @ Z(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ X(11)) + 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Y(10) @ Z(13)) + 0.010540430289943614 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ X(10) @ Z(13)) + 4.183841616740977e-06 * (Y(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(12) @ Z(13)) + 4.183841616740977e-06 * (X(6) @ Z(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(12) @ Z(13)) + 0.1675666446326793 * (Z(7) @ Z(9)) + 0.11952440519292769 * (Z(7) @ Z(11)) + -1.8551275008175092e-06 * (Z(7) @ Y(11) @ Z(12) @ Y(13)) + -1.8551275008175092e-06 * (Z(7) @ X(11) @ Z(12) @ X(13)) + 0.13401730407158907 * (Z(7) @ Z(13)) + 0.18144004012596054 * (Z(7) @ Z(8)) + 0.029812336059742324 * (Y(7) @ Z(9) @ Z(10) @ Y(11)) + 0.029812336059742324 * (X(7) @ Z(9) @ Z(10) @ X(11)) + -3.2774327636709167e-06 * (Y(7) @ Z(9) @ Z(10) @ Z(11) @ Z(12) @ Y(13)) + -3.2774327636709167e-06 * (X(7) @ Z(9) @ Z(10) @ Z(11) @ Z(12) @ X(13)) + 0.0002922181191170979 * (Y(7) @ X(8) @ X(9) @ Y(10)) + -0.0002922181191170979 * (Y(7) @ Y(8) @ X(9) @ X(10)) + -0.0002922181191170979 * (X(7) @ X(8) @ Y(9) @ Y(10)) + 0.0002922181191170979 * (X(7) @ Y(8) @ Y(9) @ X(10)) + -3.3280759108072957e-07 * (Y(7) @ X(8) @ X(9) @ Z(10) @ Z(11) @ Y(12)) + 3.3280759108072957e-07 * (Y(7) @ Y(8) @ X(9) @ Z(10) @ Z(11) @ X(12)) + 3.3280759108072957e-07 * (X(7) @ X(8) @ Y(9) @ Z(10) @ Z(11) @ Y(12)) + -3.3280759108072957e-07 * (X(7) @ Y(8) @ Y(9) @ Z(10) @ Z(11) @ X(12)) + 0.030104554178859426 * (Y(7) @ Z(8) @ Z(10) @ Y(11)) + 0.030104554178859426 * (X(7) @ Z(8) @ Z(10) @ X(11)) + -3.6102403547517547e-06 * (Y(7) @ Z(8) @ Z(10) @ Z(11) @ Z(12) @ Y(13)) + -3.6102403547517547e-06 * (X(7) @ Z(8) @ Z(10) @ Z(11) @ Z(12) @ X(13)) + 0.13734945522934094 * (Z(7) @ Z(10)) + 0.011307228315219147 * (Y(7) @ Z(8) @ Z(9) @ Y(11)) + 0.011307228315219147 * (X(7) @ Z(8) @ Z(9) @ X(11)) + -6.5242355753560775e-06 * (Y(7) @ Z(8) @ Z(9) @ Z(11) @ Z(12) @ Y(13)) + -6.5242355753560775e-06 * (X(7) @ Z(8) @ Z(9) @ Z(11) @ Z(12) @ X(13)) + -2.890941037649085e-06 * (Z(7) @ Y(10) @ Z(11) @ Y(12)) + -2.890941037649085e-06 * (Z(7) @ X(10) @ Z(11) @ X(12)) + 3.3130491730399857e-06 * (Y(7) @ Z(8) @ Z(9) @ X(10) @ X(11) @ Y(12)) + -3.3130491730399857e-06 * (Y(7) @ Z(8) @ Z(9) @ Y(10) @ X(11) @ X(12)) + -3.3130491730399857e-06 * (X(7) @ Z(8) @ Z(9) @ X(10) @ Y(11) @ Y(12)) + 3.3130491730399857e-06 * (X(7) @ Z(8) @ Z(9) @ Y(10) @ Y(11) @ X(12)) + -0.014564491580696262 * (Y(7) @ Z(8) @ Z(9) @ X(10) @ X(12) @ Y(13)) + -0.014564491580696262 * (Y(7) @ Z(8) @ Z(9) @ Y(10) @ Y(12) @ Y(13)) + -0.014564491580696262 * (X(7) @ Z(8) @ Z(9) @ X(10) @ X(12) @ X(13)) + -0.014564491580696262 * (X(7) @ Z(8) @ Z(9) @ Y(10) @ Y(12) @ X(13)) + -3.211186402316478e-06 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Z(12) @ Y(13)) + -3.211186402316478e-06 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ Z(12) @ X(13)) + 0.025104921870639875 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11) @ Z(13)) + 0.025104921870639875 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ X(11) @ Z(13)) + 0.1513833780524887 * (Z(7) @ Z(12)) + 0.010540430289943614 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Y(11) @ Z(12)) + 0.010540430289943614 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ X(11) @ Z(12)) + 4.183841616740977e-06 * (Y(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ Y(13)) + 4.183841616740977e-06 * (X(7) @ Z(8) @ Z(9) @ Z(10) @ Z(11) @ X(13)) + 0.1376686338096208 * (Z(8) @ Z(10)) + -1.597330366518286e-06 * (Z(8) @ Y(10) @ Z(11) @ Y(12)) + -1.597330366518286e-06 * (Z(8) @ X(10) @ Z(11) @ X(12)) + 0.14973493699385057 * (Z(8) @ Z(12)) + 0.2200397733437613 * (Z(8) @ Z(9)) + 0.0095607137731044 * (Y(8) @ X(9) @ X(10) @ Y(11)) + -0.0095607137731044 * (Y(8) @ Y(9) @ X(10) @ X(11)) + -0.0095607137731044 * (X(8) @ X(9) @ Y(10) @ Y(11)) + 0.0095607137731044 * (X(8) @ Y(9) @ Y(10) @ X(11)) + 6.628464327049607e-07 * (Y(8) @ X(9) @ X(11) @ Y(12)) + 6.628464327049607e-07 * (Y(8) @ Y(9) @ Y(11) @ Y(12)) + 6.628464327049607e-07 * (X(8) @ X(9) @ X(11) @ X(12)) + 6.628464327049607e-07 * (X(8) @ Y(9) @ Y(11) @ X(12)) + -6.628464327049607e-07 * (Y(8) @ X(9) @ X(10) @ Z(11) @ Z(12) @ Y(13)) + 6.628464327049607e-07 * (Y(8) @ Y(9) @ X(10) @ Z(11) @ Z(12) @ X(13)) + 6.628464327049607e-07 * (X(8) @ X(9) @ Y(10) @ Z(11) @ Z(12) @ Y(13)) + -6.628464327049607e-07 * (X(8) @ Y(9) @ Y(10) @ Z(11) @ Z(12) @ X(13)) + 0.006087832272267014 * (Y(8) @ X(9) @ X(12) @ Y(13)) + -0.006087832272267014 * (Y(8) @ Y(9) @ X(12) @ X(13)) + -0.006087832272267014 * (X(8) @ X(9) @ Y(12) @ Y(13)) + 0.006087832272267014 * (X(8) @ Y(9) @ Y(12) @ X(13)) + 0.1472293475827252 * (Z(8) @ Z(11)) + -9.34483933813339e-07 * (Z(8) @ Y(11) @ Z(12) @ Y(13)) + -9.34483933813339e-07 * (Z(8) @ X(11) @ Z(12) @ X(13)) + 0.1558227692661176 * (Z(8) @ Z(13)) + 0.1376686338096208 * (Z(9) @ Z(11)) + -1.597330366518286e-06 * (Z(9) @ Y(11) @ Z(12) @ Y(13)) + -1.597330366518286e-06 * (Z(9) @ X(11) @ Z(12) @ X(13)) + 0.14973493699385057 * (Z(9) @ Z(13)) + 0.1472293475827252 * (Z(9) @ Z(10)) + -9.34483933813339e-07 * (Z(9) @ Y(10) @ Z(11) @ Y(12)) + -9.34483933813339e-07 * (Z(9) @ X(10) @ Z(11) @ X(12)) + 0.1558227692661176 * (Z(9) @ Z(12)) + 0.11270383378135919 * (Z(10) @ Z(12)) + 0.14926349629547572 * (Z(10) @ Z(11)) + -8.194129406674639e-06 * (Y(10) @ Y(12)) + -8.194129406674639e-06 * (X(10) @ X(12)) + -8.194129406674639e-06 * (Z(10) @ Y(11) @ Z(12) @ Y(13)) + -8.194129406674639e-06 * (Z(10) @ X(11) @ Z(12) @ X(13)) + 0.028685206654421494 * (Y(10) @ X(11) @ X(12) @ Y(13)) + -0.028685206654421494 * (Y(10) @ Y(11) @ X(12) @ X(13)) + -0.028685206654421494 * (X(10) @ X(11) @ Y(12) @ Y(13)) + 0.028685206654421494 * (X(10) @ Y(11) @ Y(12) @ X(13)) + 0.14138904043578068 * (Z(10) @ Z(13)) + 7.954260900515966e-06 * (Y(10) @ Z(11) @ Y(12) @ Z(13)) + 7.954260900515966e-06 * (X(10) @ Z(11) @ X(12) @ Z(13)) + 0.11270383378135919 * (Z(11) @ Z(13)) + 0.14138904043578068 * (Z(11) @ Z(12)) + 7.954260900515966e-06 * (Y(11) @ Y(13)) + 7.954260900515966e-06 * (X(11) @ X(13)) + 0.15435756308747034 * (Z(12) @ Z(13))

This backend requires the OpenFermion-PySCF plugin to be installed by the user with

pip install openfermionpyscf

Additionally, if you have built your electronic Hamiltonian independently using OpenFermion tools, it can be readily converted to a PennyLane observable using the import_operator() function.

You have completed the tutorial! Now, select your favorite molecule and build its electronic Hamiltonian. To see how simple it is to implement the VQE algorithm to compute the ground-state energy of your molecule using PennyLane, take a look at the tutorial demos/tutorial_vqe.

References

1

Yudong Cao, Jonathan Romero, et al., “Quantum Chemistry in the Age of Quantum Computing”. Chem. Rev. 2019, 119, 19, 10856-10915.

2

M. Born, J.R. Oppenheimer, “Quantum Theory of the Molecules”. Annalen der Physik 84, 457-484 (1927)

3

Rolf Seeger, John Pople. “Self‐consistent molecular orbital methods. XVIII. Constraints and stability in Hartree–Fock theory”. Journal of Chemical Physics 66, 3045 (1977).

4

J.T. Fermann, E.F. Valeev, “Fundamentals of Molecular Integrals Evaluation”. arXiv:2007.12057

5

Jacob T. Seeley, Martin J. Richard, Peter J. Love. “The Bravyi-Kitaev transformation for quantum computation of electronic structure”. Journal of Chemical Physics 137, 224109 (2012).

6

J.J. Bao, S.S. Dong, L. Gagliardi, D.G. Truhlar. “Automatic Selection of an Active Space for Calculating Electronic Excitation Spectra by MS-CASPT2 or MC-PDFT”. Journal of Chemical Theory and Computation 14, 2017 (2018).

About the author

Alain Delgado Gran
Alain Delgado Gran

Alain Delgado Gran

Quantum simulations of molecules and materials.

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Using PennyLane with PySCF and OpenFermion

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VQE in different spin sectors

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Qubit tapering

Adaptive circuits for quantum chemistry

Mapping fermionic Hamiltonians to qubit Hamiltonians

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